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RESONANT ANISOTROPIC EMISSION IN RABBITT SPECTROSCOPY

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Date Issued:
2018
Abstract/Description:
A variant of RABBITT pump-probe spectroscopy in which the attosecond pulse train comprises both even and odd harmonics of the fundamental IR probe frequency is explored to measure time-resolved photoelectron emission in systems that exhibit autoionizing states. It is shown that the group delay of both one-photon and two-photon resonant transitions is directly encoded in the energy-resolved photoelectron anisotropy as a function of the pump-probe time-delay. This principle is illustrated for a 1D model with symmetric zero-range potentials that supports both bound states and shape-resonances. The model is studied using both perturbation theory and solving the time-dependent Schodinger equation on a grid. Moreover, we study the case of a realistic atomic system, helium. In both cases, we demonstrate faithful reconstruction of the phase information for resonant photoemission.
Title: RESONANT ANISOTROPIC EMISSION IN RABBITT SPECTROSCOPY.
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Name(s): Ghomashi, Bejan M, Author
Argenti, Luca, Committee Chair
Douguet, Nicolas, Committee Member
University of Central Florida, Degree Grantor
Type of Resource: text
Date Issued: 2018
Publisher: University of Central Florida
Language(s): English
Abstract/Description: A variant of RABBITT pump-probe spectroscopy in which the attosecond pulse train comprises both even and odd harmonics of the fundamental IR probe frequency is explored to measure time-resolved photoelectron emission in systems that exhibit autoionizing states. It is shown that the group delay of both one-photon and two-photon resonant transitions is directly encoded in the energy-resolved photoelectron anisotropy as a function of the pump-probe time-delay. This principle is illustrated for a 1D model with symmetric zero-range potentials that supports both bound states and shape-resonances. The model is studied using both perturbation theory and solving the time-dependent Schodinger equation on a grid. Moreover, we study the case of a realistic atomic system, helium. In both cases, we demonstrate faithful reconstruction of the phase information for resonant photoemission.
Identifier: CFH2000451 (IID), ucf:45703 (fedora)
Note(s): 2018-08-01
B.S.
College of Sciences, Physics
Bachelors
This record was generated from author submitted information.
Subject(s): RABBITT
spectroscopy
high-harmonic generation
ultrafast
helium
resonance
Persistent Link to This Record: http://purl.flvc.org/ucf/fd/CFH2000451
Restrictions on Access: public
Host Institution: UCF

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