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INTEGRATION OF A NANOSTRUCTURE EMBEDDED THERMORESPONSIVE POLYMER FOR MICROFLUIDIC APPLICATIONS

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Date Issued:
2008
Abstract/Description:
This work describes the modeling, synthesis, integration and characterization of a novel nanostructure embedded thermoresponsive material for microfluidic applications. The innumerable applications of thermoresponsive surfaces in the recent years have necessitated the development of a rigorous mathematical treatment for these surfaces to understand and improve their behavior. An analytical model is proposed to describe the transfer characteristic (variation of contact angle versus temperature) of a unique switchable, nanostructured, thermoresponsive surface consisting of silica nanoparticles and the thermoresponsive polymer, Poly(N-isopropylacrylamide ) (PNIPAAm) which changes its wetting angle upon heating. Important metrics such as the absolute lower critical solution temperature, threshold & saturation temperatures and gain are modeled and quantified by mathematical expressions. Based on the modeling, a heat source for the thermoresponsive surface was integrated on the glass substrate itself to create a fully functional smart surface. The design and fabrication of a smart platform consisting of the switchable, nanostructured, thermoresponsive surface with an integrated gold microheater for wettability control and its time response analysis was conducted. The insight gained into the behavior of the thermoresponsive surface by using the analytical model, aided the effort in the effective integration of the surface into a microfluidic channel for flow regulation applications. The implementations of novel microfluidic flow regulator concepts were tested. The aim is to integrate a regulator function to a channel surface utilizing the layer-by-layer (LBL) deposition technique. The characterization and pressure differential study of the microfluidic regulators was carried out on simple straight microchannels which were selectively coated with the thermoresponsive surface. Theoretical and experimental studies were performed to determine the important characteristic parameters including capillary, Weber and Reynolds numbers. The pressure differential data was used to develop critical operating specifications. This work lays out a new microfluidic device concept consisting of a channel with a built-in regulatory function.
Title: INTEGRATION OF A NANOSTRUCTURE EMBEDDED THERMORESPONSIVE POLYMER FOR MICROFLUIDIC APPLICATIONS.
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Name(s): Londe, Ghanashyam, Author
Cho, Hyoung Jin, Committee Chair
University of Central Florida, Degree Grantor
Type of Resource: text
Date Issued: 2008
Publisher: University of Central Florida
Language(s): English
Abstract/Description: This work describes the modeling, synthesis, integration and characterization of a novel nanostructure embedded thermoresponsive material for microfluidic applications. The innumerable applications of thermoresponsive surfaces in the recent years have necessitated the development of a rigorous mathematical treatment for these surfaces to understand and improve their behavior. An analytical model is proposed to describe the transfer characteristic (variation of contact angle versus temperature) of a unique switchable, nanostructured, thermoresponsive surface consisting of silica nanoparticles and the thermoresponsive polymer, Poly(N-isopropylacrylamide ) (PNIPAAm) which changes its wetting angle upon heating. Important metrics such as the absolute lower critical solution temperature, threshold & saturation temperatures and gain are modeled and quantified by mathematical expressions. Based on the modeling, a heat source for the thermoresponsive surface was integrated on the glass substrate itself to create a fully functional smart surface. The design and fabrication of a smart platform consisting of the switchable, nanostructured, thermoresponsive surface with an integrated gold microheater for wettability control and its time response analysis was conducted. The insight gained into the behavior of the thermoresponsive surface by using the analytical model, aided the effort in the effective integration of the surface into a microfluidic channel for flow regulation applications. The implementations of novel microfluidic flow regulator concepts were tested. The aim is to integrate a regulator function to a channel surface utilizing the layer-by-layer (LBL) deposition technique. The characterization and pressure differential study of the microfluidic regulators was carried out on simple straight microchannels which were selectively coated with the thermoresponsive surface. Theoretical and experimental studies were performed to determine the important characteristic parameters including capillary, Weber and Reynolds numbers. The pressure differential data was used to develop critical operating specifications. This work lays out a new microfluidic device concept consisting of a channel with a built-in regulatory function.
Identifier: CFE0002368 (IID), ucf:47786 (fedora)
Note(s): 2008-12-01
Ph.D.
Engineering and Computer Science, School of Electrical Engineering and Computer Science
Doctorate
This record was generated from author submitted information.
Subject(s): Thermoresponsive
PNIPAAm
Nanostructure
Layer-by-Layer
Logistic function
Microfluidic flow regulation
Pressure differential
Persistent Link to This Record: http://purl.flvc.org/ucf/fd/CFE0002368
Restrictions on Access: public
Host Institution: UCF

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