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Size, Shape, Composition and Chemical state effects in nanocatalysis

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Date Issued:
2016
Abstract/Description:
The field of nanocatalysis has gained significant attention in the last decades due to the numerous industrial applications of nanosized catalysts. Size, shape, structure, and composition of the nanoparticles (NPs) are the parameters that can affect the reactivity, selectivity and stability of nanocatalysts. Therefore, understanding how these parameters affect the catalytic properties of these systems is required in order to engineer them with a given desired performance. It is also important to gain insight into the structural evolution of the NP catalysts under different reaction conditions to design catalysts with long durability under reaction condition. In this dissertation a synergistic combination of in situ, ex situ and operando state-of-the art techniques have allowed me to explore a variety of parameters and phenomena relevant to nanocatalysts by systematically tuning the NP size, chemical state, composition and chemical environment.
Title: Size, Shape, Composition and Chemical state effects in nanocatalysis.
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Name(s): Ahmadi, Mahdi, Author
Roldan Cuenya, Beatriz, Committee Chair
Rahman, Talat, Committee Member
Kara, Abdelkader, Committee Member
Coffey, Kevin, Committee Member
University of Central Florida, Degree Grantor
Type of Resource: text
Date Issued: 2016
Publisher: University of Central Florida
Language(s): English
Abstract/Description: The field of nanocatalysis has gained significant attention in the last decades due to the numerous industrial applications of nanosized catalysts. Size, shape, structure, and composition of the nanoparticles (NPs) are the parameters that can affect the reactivity, selectivity and stability of nanocatalysts. Therefore, understanding how these parameters affect the catalytic properties of these systems is required in order to engineer them with a given desired performance. It is also important to gain insight into the structural evolution of the NP catalysts under different reaction conditions to design catalysts with long durability under reaction condition. In this dissertation a synergistic combination of in situ, ex situ and operando state-of-the art techniques have allowed me to explore a variety of parameters and phenomena relevant to nanocatalysts by systematically tuning the NP size, chemical state, composition and chemical environment.
Identifier: CFE0006243 (IID), ucf:51084 (fedora)
Note(s): 2016-08-01
Ph.D.
Sciences, Physics
Doctoral
This record was generated from author submitted information.
Subject(s): Nanoparticles -- heterogeneous catalysis -- Nanocatalysis -- Bimetallic -- Support interaction
Persistent Link to This Record: http://purl.flvc.org/ucf/fd/CFE0006243
Restrictions on Access: public 2016-08-15
Host Institution: UCF

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