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Title: Filament Plasma Density Enhancement Using Two Co-Propagating Beams.
Creator: Pena, Jessica, Richardson, Martin, Moharam, Jim, Gaume, Romain, Rostami Fairchild, Shermineh, University of Central Florida
Abstract / Description: Filaments are self-guided plasma channels generated from laser pulses with power above a critical value. They can propagate several times the Rayleigh length for diffraction and can travel through adverse atmospheric conditions. As such, filaments are useful in applications such as long wavelength electromagnetic and electric discharge guiding, and weather manipulation to name a few. Arrays of filaments can be useful to these applications, particularly in the generation of waveguides. However...
Show moreFilaments are self-guided plasma channels generated from laser pulses with power above a critical value. They can propagate several times the Rayleigh length for diffraction and can travel through adverse atmospheric conditions. As such, filaments are useful in applications such as long wavelength electromagnetic and electric discharge guiding, and weather manipulation to name a few. Arrays of filaments can be useful to these applications, particularly in the generation of waveguides. However, understanding the filament-induced plasma dynamics of two closely propagating beams is crucial in designing the ideal waveguide. One common way to characterize a filament is through the electron density of the plasma channel, a property which has previously been proven to be clamped for a single filament. This work will show how the electron density can be enhanced through the use of two co-propagating beams, taking advantage of their interaction. Three cases were studied: two sub-critical beams, one subcritical beam and one filament, and two filaments. The separations and focusing conditions of the beams were also varied. Enhancement of the electron density and lengthening of the plasma lifetime will be discussed for each case.
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Date Issued: 2019
Identifier: CFE0007702, ucf:52436
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0007702

Title: Design and Engineering Criteria for Optical Parametric Chirped Pulse Amplifier Systems.
Creator: Bodnar, Nathan, Richardson, Martin, Delfyett, Peter, Likamwa, Patrick, Baudelet, Matthieu, Shah, Lawrence, University of Central Florida
Abstract / Description: The generation of a quasi-single-cycle laser light pulse is a goal in many laser applications experiments. Some involve in High Harmonic Generation (HHG) and Attosecond Sciences. The demand for ultrafast laser facilities has grown; the techniques and availability of materials have changed; thereby posing new design challenges in building Optical Parametric Chirped Pulse Amplification (OPCPA) laser facilities. The concepts and challenges are discussed in detail in the development of two laser...
Show moreThe generation of a quasi-single-cycle laser light pulse is a goal in many laser applications experiments. Some involve in High Harmonic Generation (HHG) and Attosecond Sciences. The demand for ultrafast laser facilities has grown; the techniques and availability of materials have changed; thereby posing new design challenges in building Optical Parametric Chirped Pulse Amplification (OPCPA) laser facilities. The concepts and challenges are discussed in detail in the development of two laser systems within the Laser Plasma Laboratory, HERACLES and PhaSTHEUS. This dissertation also gives insight to the challenges that are encountered in other cutting edge OPCPA laser facilities. An overview of the design challenges that need to be addressed in any OPCPA laser facility either high energy or high average power that is suitable for high intensity laser physics is discussed in this dissertation.
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Date Issued: 2018
Identifier: CFE0007158, ucf:52300
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0007158

Title: Design and Engineering of Ultrafast Amplifier Systems.
Creator: Webb, Benjamin, Richardson, Martin, Chang, Zenghu, Delfyett, Peter, Gaume, Romain, Shah, Lawrence, Klemm, Richard, University of Central Florida
Abstract / Description: Recently, the design and engineering of ultrafast laser systems have led to an extraordinary increase in laser power and performance which have brought about advances in many fields such as medicine, material processing, communications, remote sensing, spectroscopy, nonlinear optics, and atomic physics. In this work, several ultrafast amplification techniques -- including chirped-pulse amplification (CPA), optical parametric chirped-pulse amplification (OPCPA), and divided-pulse amplification...
Show moreRecently, the design and engineering of ultrafast laser systems have led to an extraordinary increase in laser power and performance which have brought about advances in many fields such as medicine, material processing, communications, remote sensing, spectroscopy, nonlinear optics, and atomic physics. In this work, several ultrafast amplification techniques -- including chirped-pulse amplification (CPA), optical parametric chirped-pulse amplification (OPCPA), and divided-pulse amplification (DPA) -- are described and demonstrated in the design and construction of two ultrafast laser facilities. An existing Ti:Sapphire laser system was completely redesigned with an increased power of 10 TW for experiments capable of generating hundreds of laser filaments in ordered arrays. The performance of DPA above the Joule-level was investigated in a series of experiments utilizing various DPA schemes with gain-saturated amplifiers at high pulse energy. A new high energy OPCPA facility has been designed and its pump laser system constructed, utilizing the technique of DPA for the first time in a flashlamp-pumped amplifier chain and with a record combined energy of 5 Joules in a 230 ps pulse duration. The demonstrated OPCPA pump performance will allow for the generation of 50 TW quasi-single cycle 5 fs pulses at 2.5 Hz from a table-top OPCPA system.
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Date Issued: 2016
Identifier: CFE0006547, ucf:51349
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0006547

Title: High Energy, High Average Power, Picosecond Laser Systems to Drive Few-Cycle OPCPA.
Creator: Vaupel, Andreas, Richardson, Martin, Delfyett, Peter, Schulzgen, Axel, Shivamoggi, Bhimsen, University of Central Florida
Abstract / Description: The invention of chirped-pulse amplification (CPA) in 1985 led to a tremendous increase in obtainable laser pulse peak intensities. Since then, several table-top, Ti:sapphire-based CPA systems exceeding the 100 TW-level with more than 10 W average power have been developed and several systems are now commercially available. Over the last decade, the complementary technology of optical parametric chirped-pulse amplification (OPCPA) has improved in its performance to a competitive level. OPCPA...
Show moreThe invention of chirped-pulse amplification (CPA) in 1985 led to a tremendous increase in obtainable laser pulse peak intensities. Since then, several table-top, Ti:sapphire-based CPA systems exceeding the 100 TW-level with more than 10 W average power have been developed and several systems are now commercially available. Over the last decade, the complementary technology of optical parametric chirped-pulse amplification (OPCPA) has improved in its performance to a competitive level. OPCPA allows direct amplification of an almost-octave spanning bandwidth supporting few-cycle pulse durations at center wavelengths ranging from the visible to the mid-IR. The current record in peak power from a table-top OPCPA is 16 TW and the current record average power is 22 W. High energy, few-cycle pulses with stabilized carrier-envelope phase (CEP) are desired for applications such as high-harmonic generation (HHG) enabling attoscience and the generation keV-photon bursts.This dissertation conceptually, numerically and experimentally describes essential aspects of few-cycle OPCPA, and the associated pump beam generation. The main part of the conducted research was directed towards the few-cycle OPCPA facility developed in the Laser Plasma Laboratory at CREOL (University of Central Florida, USA) termed HERACLES. This facility was designed to generate few-cycle pulses in the visible with mJ-level pulse energy, W-level average power and more than 100 GW peak power. Major parts of the implementation of the HERACLES facility are presented.The pump generation beam of the HERACLES system has been improved in terms of pulse energy, average power and stability over the last years. It is based on diode-pumped, solid-state amplifiers with picosecond duration and experimental investigations are presented in detail. A robust system has been implemented producing mJ-level pulse energies with ~100 ps pulse duration at kHz repetition rates. Scaling of this system to high power ((>)30 W) and high peak power (50-MW-level) as well as ultra-high pulse energy ((>)160 mJ) is presented. The latter investigation resulted in the design of an ultra-high energy system for OPCPA pumping. Following this, a new OPCPA facility was designed termed PhaSTHEUS, which is anticipated to reach ultra-high intensities.Another research effort was conducted at CELIA (Univerist(&)#233; de Bordeaux 1, France) and aimed towards a previously unexplored operational regime of OPCPA with ultra-high repetition rates (10 MHz) and high average power. A supercontinuum seed beam generation has been established with an output ranging from 1.3 to 1.9 ?m and few ps duration. The pump beam generation has been implemented based on rod-type fiber amplifiers producing more than 37 W average power and 370 kW peak power. The utility of this system as an OPCPA pump laser is presented along with the OPA design.The discussed systems operate in radically different regimes in terms of peak power, average power, and repetition rate. The anticipated OPCPA systems with few-cycle duration enable a wide range of novel experimental studies in attoscience, ultrafast materials processing, filamentation, LIBS and coherent control.
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Date Issued: 2013
Identifier: CFE0004952, ucf:49570
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0004952

Title: DISPERSION-MANAGED BREATHING-MODE SEMICONDUCTOR MODE-LOCKED RING LASER: EXPERIMENTAL STUDY, NUMERICAL SIMULATIONS AND APPLICATIONS.
Creator: Resan, Bojan, Delfyett, Peter J., University of Central Florida
Abstract / Description: A novel dispersion-managed breathing-mode semiconductor mode-locked ring laser is developed. The "breathing-mode" designation derives from the fact that intracavity pulses are alternately stretched and compressed as they circulate around the ring resonator. The pulses are stretched before entering the semiconductor gain medium to minimize the detrimental strong integrating self-phase modulation and to enable efficient pulse amplification. Subsequently compressed pulses facilitate bleaching...
Show moreA novel dispersion-managed breathing-mode semiconductor mode-locked ring laser is developed. The "breathing-mode" designation derives from the fact that intracavity pulses are alternately stretched and compressed as they circulate around the ring resonator. The pulses are stretched before entering the semiconductor gain medium to minimize the detrimental strong integrating self-phase modulation and to enable efficient pulse amplification. Subsequently compressed pulses facilitate bleaching the semiconductor saturable absorber. The intracavity pulse compression ratio is higher than 50. Down chirping when compared to up chirping allows broader mode-locked spectra and shorter pulse generation owing to temporal and spectral semiconductor gain dynamics. Pulses as short as 185 fs, with a peak power of ~230 w, and a focused intensity of ~4.6 gw/cm2 are generated by linear down chirp compensation and characterized by shg-frog method. To our knowledge, this is the highest peak power and the shortest pulse generation from an electrically pumped all-semiconductor system. The very good agreement between the simulated and the measured results verifies our understanding and ability to control the physical mechanisms involved in the pulse shaping within the ring cavity. Application trends such as continuum generation via a photonic crystal fiber, two-photon fluorescence imaging, and ultrafast pulse source for pump-probe experiments are demonstrated.
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Date Issued: 2004
Identifier: CFE0000176, ucf:46155
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0000176

Title: High flux isolated attosecond pulse generation.
Creator: Wu, Yi, Chang, Zenghu, Richardson, Martin, Christodoulides, Demetrios, Rahman, Talat, University of Central Florida
Abstract / Description: This thesis outlines the high intensity tabletop attosecond extreme ultraviolet laser source at the Institute for the Frontier of Attosecond Science and Technology Laboratory.First, a unique Ti:Sapphire chirped pulse amplifier laser system that delivers 14 fs pulses with 300 mJ energy at a 10 Hz repetition rate was designed and built. The broadband spectrum extending from 700 nm to 900 nm was obtained by seeding a two stage Ti:Sapphire chirped pulse power amplifier with mJ-level white light...
Show moreThis thesis outlines the high intensity tabletop attosecond extreme ultraviolet laser source at the Institute for the Frontier of Attosecond Science and Technology Laboratory.First, a unique Ti:Sapphire chirped pulse amplifier laser system that delivers 14 fs pulses with 300 mJ energy at a 10 Hz repetition rate was designed and built. The broadband spectrum extending from 700 nm to 900 nm was obtained by seeding a two stage Ti:Sapphire chirped pulse power amplifier with mJ-level white light pulses from a gas filled hollow core fiber. It is the highest energy level ever achieved by a broadband pulse in a chirped pulse amplifier up to the current date.Second, using this laser as a driving laser source, the generalized double optical gating method is employed to generate isolated attosecond pulses. Detailed gate width analysis of the ellipticity dependent pulse were performed. Calculation of electron light interaction dynamics on the atomic level was carried out to demonstrate the mechanism of isolated pulse generation.Third, a complete diagnostic apparatus was built to extract and analyze the generated attosecond pulse in spectral domain. The result confirms that an extreme ultraviolet super continuum supporting 230 as isolated attosecond pulses at 35 eV was generated using the generalized double optical gating technique. The extreme ultraviolet pulse energy was ~100 nJ at the exit of the argon gas target.
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Date Issued: 2013
Identifier: CFE0005075, ucf:49949
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0005075

Title: Phase-locking Stability of a Quasi-single-cycle Pulse.
Creator: Bodnar, Nathan, Richardson, Martin, Chang, Zenghu, Delfyett, Peter, University of Central Florida
Abstract / Description: There is increasing interest in the generation of very short laser pulses, even down to attosecond (10-18 s) durations. Laser systems with femtosecond pulse durations are needed for these applications. For many of these applications, positioning of the maximum electric field within the pulse envelope can affect the outcome. The peak of the electric field relative to the peak of the pulse is called the Carrier Envelope Phase (CEP). Controlling the position of the electric field becomes more...
Show moreThere is increasing interest in the generation of very short laser pulses, even down to attosecond (10-18 s) durations. Laser systems with femtosecond pulse durations are needed for these applications. For many of these applications, positioning of the maximum electric field within the pulse envelope can affect the outcome. The peak of the electric field relative to the peak of the pulse is called the Carrier Envelope Phase (CEP). Controlling the position of the electric field becomes more important when pulse duration approaches single-cycle.This thesis focuses on the stabilization of a quasi-single-cycle laser facility. Improvements to this already-established laser facility, HERACLES (High Energy, Repetition rate Adjustable, Carrier-Locked-to-Envelope System) described in this thesis include a stabilized pump line and the improvement in CEP stabilization electronics. HERACLES is built upon an Optical Parametric Chirped Pulse Amplification (OPCPA) architecture. This architecture uses Optical Parametric Amplification (OPA) as the gain material to increase the output energy of the system. OPA relies on a nonlinear process to generate high gain (106) with ultra-wide bandwidth. Instabilities in the OPA driving pump energy can create dynamically fluctuations in the final OPCPA output energy. To reduce these fluctuations two key upgrades were implemented on the pump beam. Both were major improvements in the stability. Firstly, an improved regenerative amplifier design reduced beam pointing fluctuations. Secondly, the addition of a pump monitoring system with feedback-control eliminated long-term power drifts. Both enhanced the OPA pulse-to-pulse and long-term stability.To improve the stability in measuring CEP drifts, modification of the feedback electronics was needed. The modification consisted of integrating noise reduction electronics. This novel noise reducer uses a similar process to a super-heterodyne receiver. The noise reducer resulted in 60 dB reduction of out-of-band noise. This led to increased signal quality with cleaner amplification of weaker signals. The enhanced signal quality led to more reliable long-term locking. The synthetically increased signal-to-noise ratio allows locking of the CEP frequency below the typically requirements. This integration allows relaxed constraints on the laser systems.The optics and electronics of a high-power, quasi-single cycle laser facility were improved. This thesis included the stabilization of the pump line and the stabilization of the CEP. This work allows for new long-duration experiments.
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Date Issued: 2013
Identifier: CFE0004654, ucf:49908
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0004654

Title: THE EFFECTS OF ELECTRODE GEOMETRY ON CURRENT PULSE CAUSED BY ELECTRICAL DISCHARGE OVER AN ULTRA-FAST LASER FILAMENT.
Creator: Bubelnik, Matthew, Siders, Craig, University of Central Florida
Abstract / Description: The time-resolved electrical conductivity of a short-pulse generated plasma filament in air was studied. Close-coupled metal electrodes were used to discharge the stored energy of a high-voltage capacitor and the resulting microsecond-scale electrical discharge was measured using fast current sensors. Significant differences in the time dependence of the current were seen with the two electrode geometries used. Using sharp-tipped electrodes additional peaks in the time-resolved conductivity...
Show moreThe time-resolved electrical conductivity of a short-pulse generated plasma filament in air was studied. Close-coupled metal electrodes were used to discharge the stored energy of a high-voltage capacitor and the resulting microsecond-scale electrical discharge was measured using fast current sensors. Significant differences in the time dependence of the current were seen with the two electrode geometries used. Using sharp-tipped electrodes additional peaks in the time-resolved conductivity were seen, relative to the single peak seen with spherical electrodes. We attribute these additional features to secondary electron collisional ionization brought about by field enhancement at the tips. Additional discrepancies in the currents measured leaving the high-voltage electrode and that returning to ground were also observed. Implications for potential laser-induced discharge applications will be discussed.
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Date Issued: 2005
Identifier: CFE0000447, ucf:46378
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0000447

Title: Towards High-Flux Isolated Attosecond Pulses with a 200 TW CPA.
Creator: Cunningham, Eric, Chang, Zenghu, Saleh, Bahaa, Soileau, MJ, Saha, Haripada, University of Central Florida
Abstract / Description: Attosecond pulses have been developed as a means for investigating phenomena that proceed on the order of the atomic unit of time (24 as). Unfortunately, these extreme ultraviolet (XUV) pulses by themselves contain too few photons to initiate nonlinear dynamics or dress states in an attosecond pump--attosecond probe scheme. As a result, most attosecond experiments thus far have featured complementary near infrared (NIR) femtosecond lasers for instigating electron dynamics. In order to access...
Show moreAttosecond pulses have been developed as a means for investigating phenomena that proceed on the order of the atomic unit of time (24 as). Unfortunately, these extreme ultraviolet (XUV) pulses by themselves contain too few photons to initiate nonlinear dynamics or dress states in an attosecond pump--attosecond probe scheme. As a result, most attosecond experiments thus far have featured complementary near infrared (NIR) femtosecond lasers for instigating electron dynamics. In order to access the benefits of all-attosecond measurements and open attosecond physics to new fields of exploration, the photon flux of these pulses must be increased.One way to boost the attosecond pulse energy is to scale up the energy of the NIR pulse responsible for driving high-harmonic generation (HHG). With generalized double optical gating (GDOG), isolated attosecond pulses can be generated with multi-cycle laser systems, wherein the pulse energy can be boosted more easily than in the few-cycle laser systems required by other gating methods. At the Institute for the Frontier of Attosecond Science and Technology (IFAST), this scalability was demonstrated using a 350 mJ, 15 fs (10 TW) Ti:sapphire laser, which was used to generate a 100 nJ XUV continuum. This represented an order-of-magnitude improvement over typical attosecond pulse energies achievable by millijoule-level few-cycle lasers.To obtain the microjoule-level attosecond pulse energy required for performing all-attosecond experiments, the attosecond flux generated by the IFAST 10 TW system was still deficient by an order of magnitude. To this end, the laser system was upgraded to provide joule-level output energies while maintaining pulse compression to 15 fs, with a targeted peak power of 200 TW. This was accomplished by adding an additional Ti:sapphire amplifier to the existing 10 TW system and implementing a new pulse compression system to accommodate the higher pulse energy.Because this system operated at a 10 Hz repetition rate, stabilization of the carrier-envelope phase (CEP) -- important for controlling attosecond pulse production -- could not be achieved using traditional methods. Therefore, a new scheme was developed, demonstrating the first-ever control of CEP in a chirped-pulse amplifier (CPA) at low repetition rates.Finally, a new variation of optical gating was proposed as a way to improve the efficiency of the attosecond pulse generation process. This method was also predicted to allow for the generation of isolated attosecond pulses with longer driving laser pulses, as well as the extension of the high-energy photon cut-off of the XUV continuum.
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Date Issued: 2015
Identifier: CFE0005938, ucf:50804
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0005938

Title: Characterization and Application of Isolated Attosecond Pulses.
Creator: Chini, Michael, Chang, Zenghu, Saha, Haripada, Chow, Lee, Schulzgen, Axel, University of Central Florida
Abstract / Description: Tracking and controlling the dynamic evolution of matter under the influence of external fields is among the most fundamental goals of physics. In the microcosm, the motion of electrons follows the laws of quantum mechanics and evolves on the timescale set by the atomic unit of time, 24 attoseconds. While only a few time-dependent quantum mechanical systems can be solved theoretically, recent advances in the generation, characterization, and application of isolated attosecond pulses and few...
Show moreTracking and controlling the dynamic evolution of matter under the influence of external fields is among the most fundamental goals of physics. In the microcosm, the motion of electrons follows the laws of quantum mechanics and evolves on the timescale set by the atomic unit of time, 24 attoseconds. While only a few time-dependent quantum mechanical systems can be solved theoretically, recent advances in the generation, characterization, and application of isolated attosecond pulses and few-cycle femtosecond lasers have given experimentalists the necessary tools for dynamic measurements on these systems. However, pioneering studies in attosecond science have so far been limited to the measurement of free electron dynamics, which can in most cases be described approximately using classical mechanics. Novel tools and techniques for studying bound states of matter are therefore desired to test the available theoretical models and to enrich our understanding of the quantum world on as-yet unprecedented timescales.In this work, attosecond transient absorption spectroscopy with ultrabroadband attosecond pulses is presented as a technique for direct measurement of electron dynamics in quantum systems, demonstrating for the first time that the attosecond transient absorption technique allows for state-resolved and simultaneous measurement of bound and continuum state dynamics. The helium atom is the primary target of the presented studies, owing to its accessibility to theoretical modeling with both ab initio simulations and to model systems with reduced dimensionality. In these studies, ultrafast dynamics (-) on timescales shorter than the laser cycle (-) are observed in prototypical quantum mechanical processes such as the AC Stark and ponderomotive energy level shifts, Rabi oscillations and electromagnetically-induced absorption and transparency, and two-color multi-photon absorption to (")dark(") states of the atom. These features are observed in both bound states and quasi-bound autoionizing states of the atom. Furthermore, dynamic interference oscillations, corresponding to quantum path interferences involving bound and free electronic states of the atom, are observed for the first time in an optical measurement. These first experiments demonstrate the applicability of attosecond transient absorption spectroscopy with ultrabroadband attosecond pulses to the study and control of electron dynamics in quantum mechanical systems with high fidelity and state selectivity. The technique is therefore ideally suited for the study of charge transfer and collective electron motion in more complex systems.The transient absorption studies on atomic bound states require ultrabroadband attosecond pulses ? attosecond pulses with large spectral bandwidth compared to their central frequency. This is due to the fact that the bound states in which we are interested lie only 15-25 eV above the ground state, so the central frequency of the pulse should lie in this range. On the other hand, the bandwidth needed to generate an isolated 100 as pulse exceeds 18 eV (-) comparable to or even larger than the central frequency. However, current methods for characterizing attosecond pulses require that the attosecond pulse spectrum bandwidth is small compared to its central frequency, known as the central momentum approximation. We therefore explore the limits of attosecond pulse characterization using the current technology and propose a novel method for characterizing ultrabroadband attosecond pules, which we term PROOF (phase retrieval by omega oscillation filtering). We demonstrate the PROOF technique with both simulated and experimental data, culminating in the characterization of a world-record-breaking 67 as pulse.
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Date Issued: 2012
Identifier: CFE0004781, ucf:49802
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0004781

Title: Generation and Characterization of Isolated Attosecond Pulse in the Soft X-ray Regime.
Creator: Li, Jie, Chang, Zenghu, Delfyett, Peter, Vanstryland, Eric, Chen, Bo, University of Central Florida
Abstract / Description: The observation of any atomic and molecular dynamics requires a probe that has a timescale comparable to the dynamics itself. Ever since the invention of laser, the temporal duration of the laser pulse has been incrementally reduced from several nanoseconds to just attoseconds. Picosecond and femtosecond laser pulses have been widely used to study molecular rotation and vibration. In 2001, the first single isolated attosecond pulse (1 attosecond = 10^-18 seconds.) was demonstrated. Since this...
Show moreThe observation of any atomic and molecular dynamics requires a probe that has a timescale comparable to the dynamics itself. Ever since the invention of laser, the temporal duration of the laser pulse has been incrementally reduced from several nanoseconds to just attoseconds. Picosecond and femtosecond laser pulses have been widely used to study molecular rotation and vibration. In 2001, the first single isolated attosecond pulse (1 attosecond = 10^-18 seconds.) was demonstrated. Since this breakthrough, (")attoscience(") has become a hot topic in ultrafast physics. Attosecond pulses typically have span between EUV to X-ray photon energies and sub-femtosecond pulse duration. It becomes an ideal tool for experimentalists to study ultrafast electron dynamics in atoms, molecules and condensed matter. The conventional scheme for generating attosecond pulses is focusing an intense femtosecond laser pulse into inert gases. The bound electrons are ionized into continuum through tunneling ionization under the strong electrical field. After ionization, the free electron will be accelerated by the laser field away from the parent ion and then recombined with its parent ion and releases its kinetic energy as a photon burst that lasts for a few hundred attoseconds. According to the classical (")three-step model("), high order harmonic will have a higher cutoff photon energy when driven by a longer wavelength laser field. Compared to Ti:sapphire lasers center at a wavelength of 800 nm, an optical parametric amplifier could offer a broad bandwidth at infrared range, which could support few cycle pulses for driving high harmonic generation in the X-ray spectrum range. In this work, an optical parametric chirped-pulse amplification system was developed to deliver CEP-stable 3-mJ, 12-fs pulses centered at 1.7 micron. We implement a chirped-pump technique to phase match the board parametric amplification bandwidth with high conversion efficiency. Using such a laser source, isolated attosecond pulses with photon exceeding 300 eV are achieved by applying the polarization gating technique at 1.7 micron. The intrinsic positive chirp of the attosecond pulses is measured by the attosecond streak camera and retrieved with our PROOF technique. Sn metal filters with negative dispersion were chosen to compensate the intrinsic attochirp. As a result, isolated 53-attosecond soft x-ray pulses are achieved. Such water window attosecond source will be a powerful tool for studying charge distribution/migration in bio-molecules and will bring opportunities to study high field physics or attochemistry.
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Date Issued: 2018
Identifier: CFE0007040, ucf:52007
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0007040

Title: Plasma Dynamics of Laser Filaments.
Creator: Reyes, Danielle, Richardson, Martin, Gaume, Romain, Chini, Michael, University of Central Florida
Abstract / Description: Laser filamentation is a complex phenomenon occurring for pulses with peak power above a critical value. A filament is a dynamic self-guided structure characterized by several unique qualities, which include a beam with a high-intensity core surrounded by an energy reservoir, a weakly ionized plasma channel, and supercontinuum generation. Several of the proposed applications for filamentation utilize the plasma channel, such as for assisted electric discharge and microwave guiding. However,...
Show moreLaser filamentation is a complex phenomenon occurring for pulses with peak power above a critical value. A filament is a dynamic self-guided structure characterized by several unique qualities, which include a beam with a high-intensity core surrounded by an energy reservoir, a weakly ionized plasma channel, and supercontinuum generation. Several of the proposed applications for filamentation utilize the plasma channel, such as for assisted electric discharge and microwave guiding. However, filament properties are highly influenced by the physical conditions under which they are formed. A host of studies have been conducted to further characterize filaments, but much work still remains in order to understand their complex behavior. This work presents an accurate and direct measurement of the electron density based on an interferometric technique. The impact of different initial parameters on filament spatio-temporal dynamics in air is investigated, concentrating primarily on their influence on the plasma. For comparison of the experiment with theory, the plasma decay is modeled by a system of kinetic equations that takes into account three-body and dissociative electron recombination reactions.
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Date Issued: 2017
Identifier: CFE0006646, ucf:51222
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0006646

Title: Dynamic feedback pulse shaping for high power chirped pulse amplification system.
Creator: Nguyen, Dat, Delfyett, Peter, Rahman, Talat, Richardson, Martin, Schulzgen, Axel, Li, Guifang, University of Central Florida
Abstract / Description: The topic of this proposal is the development of high peak power laser sources with a focus on linearly chirped pulse laser sources. In the past decade chirped optical pulses have found a plethora of applications such as photonic analog-to-digital conversion, optical coherence tomography, laser ranging, etc. This dissertation analyzes the aforementioned applications of linearly chirped pulses and their technical requirements, as well as the performance of previously demonstrated parabolic...
Show moreThe topic of this proposal is the development of high peak power laser sources with a focus on linearly chirped pulse laser sources. In the past decade chirped optical pulses have found a plethora of applications such as photonic analog-to-digital conversion, optical coherence tomography, laser ranging, etc. This dissertation analyzes the aforementioned applications of linearly chirped pulses and their technical requirements, as well as the performance of previously demonstrated parabolic pulse shaping approaches. The experimental research addresses the topic of parabolic pulse generation in two distinct ways. First, pulse shaping technique involving a time domain approach is presented, that results in stretched pulses with parabolic profiles with temporal duration of 15 ns. After pulse is shaped into a parabolic intensity profile, the pulse is compressed with DCF fiber spool by 100 times to 80 ps duration at FWHM. A different approach of pulse shaping in frequency domain is performed, in which a spectral processor based on Liquid Crystal on Silicon technology is used. The pulse is stretched to 1.5 ns before intensity mask is applied, resulting in a parabolic intensity profile. Due to frequency to time mapping, its temporal profile is also parabolic. After pulse shaping, the pulse is compressed with a bulk compressor, and subsequently analyzed with a Frequency Resolved Optical Gating (FROG). The spectral content of the compressed pulse is feedback to the spectral processor and used to adjust the spectral phase mask applied on the pulse. The resultant pulse after pulse shaping with feedback mechanism is a Fourier transform, sub-picosecond ultrashort pulse with 5 times increase in peak power.The appendices in this dissertation provide additional material used for the realization of the main research focus of the dissertation. Specification and characterization of major components of equipment and devices used in the experiment are present. The description of Matlab algorithms that was used to calculate required signals for pulse shaping are shown. A brief description of the Labview code used to control the spectral processor will also be illustrated.
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Date Issued: 2013
Identifier: CFE0004899, ucf:49642
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0004899

Title: HIGH-INTENSITY ULTRA-FAST LASER INTERACTION TECHNOLOGIES.
Creator: Bernath, Robert, Richardson, Martin, University of Central Florida
Abstract / Description: To our knowledge this is the first comprehensive study of laser-induced effects generated at intermediate distances using self-channeled femtosecond laser pulses. Studies performed were made both experimentally and theoretically with the use of novel modeling techniques. Peak laser pulse powers above 3 GW allow beam propagation without divergence for up to several kilometers. In this regime, experiments were performed at 30 meters from the laser system in a custom propagation and target range...
Show moreTo our knowledge this is the first comprehensive study of laser-induced effects generated at intermediate distances using self-channeled femtosecond laser pulses. Studies performed were made both experimentally and theoretically with the use of novel modeling techniques. Peak laser pulse powers above 3 GW allow beam propagation without divergence for up to several kilometers. In this regime, experiments were performed at 30 meters from the laser system in a custom propagation and target range, utilizing the Laser Plasma Laboratory's Terawatt laser system. Experiments included investigations of laser ablation; electromagnetic pulsed (EMP) radiation generation over the 1-18 GHz region; shockwave formation in air and solid media; optical coupling of channeled pulses into transparent media; and, conservation of energy in these interactions. The use of bursts of femtosecond pulses was found to increase the ablation rate significantly over single-pulse ablation in both air and vacuum. EMP generation from near-field focused and distance-propagated pulses was investigated. Field strengths upwards of 400 V/m/λ for vacuum focusing and 25 V/m/λ for self-channeled pulses were observed. The total field strengths over 1-18 GHz measured at distance surpassed 12 kV/m. Shockwaves generated in transparent media at 30 meters were observed as a function of time. It was found that the interaction conditions control the formation and propagation of the shock fronts into the medium. Due to the processes involved in self-channeling, significant fractions of the laser pulse were coupled into the target materials, resulting in internal optical and exit-surface damage. Basic estimations on the conservation of energy in the interaction are presented. The results of the experiments are supported by hydrodynamic plasma physics code and acoustic modeling.
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Date Issued: 2007
Identifier: CFE0001902, ucf:47497
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0001902

Title: ALL-SEMICONDUCTOR HIGH POWER MODE-LOCKED LASER SYSTEM.
Creator: Kim, Kyungbum, Delfyett, Peter, University of Central Florida
Abstract / Description: The objective of this dissertation is to generate high power ultrashort optical pulses from an all-semiconductor mode-locked laser system. The limitations of semiconductor optical amplifier in high energy, ultrashort pulse amplification are reviewed. A method to overcome the fundamental limit of small stored energy inside semiconductor optical amplifier called "eXtreme Chirped Pulse Amplification (X-CPA)" is proposed and studied theoretically and experimentally. The key benefits of the...
Show moreThe objective of this dissertation is to generate high power ultrashort optical pulses from an all-semiconductor mode-locked laser system. The limitations of semiconductor optical amplifier in high energy, ultrashort pulse amplification are reviewed. A method to overcome the fundamental limit of small stored energy inside semiconductor optical amplifier called "eXtreme Chirped Pulse Amplification (X-CPA)" is proposed and studied theoretically and experimentally. The key benefits of the concept of X-CPA are addressed. Based on theoretical and experimental study, an all-semiconductor mode-locked X-CPA system consisting of a mode-locked master oscillator, an optical pulse pre-stretcher, a semiconductor optical amplifier (SOA) pulse picker, an extreme pulse stretcher/compressor, cascaded optical amplifiers, and a bulk grating compressor is successfully demonstrated and generates >kW record peak power. A potential candidate for generating high average power from an X-CPA system, novel grating coupled surface emitting semiconductor laser (GCSEL) devices, are studied experimentally. The first demonstration of mode-locking with GCSELs and associated amplification characteristics of grating coupled surface emitting SOAs will be presented. In an effort to go beyond the record setting results of the X-CPA system, a passive optical cavity amplification technique in conjunction with the X-CPA system is constructed, and studied experimentally and theoretically.
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Date Issued: 2006
Identifier: CFE0001069, ucf:46767
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0001069

Title: Engineering and Application of Ultrafast Laser Pulses and Filamentation in Air.
Creator: Barbieri, Nicholas, Richardson, Martin, University of Central Florida
Abstract / Description: Continuing advances in laser and photonic technology has seen the development of lasers with increasing power and increasingly short pulsewidths, which have become available over an increasing range of wavelengths. As the availability of laser sources grow, so do their applications. To make better use of this improving technology, understanding and controlling laser propagation in free space is critical, as is understanding the interaction between laser light and matter.The need to better...
Show moreContinuing advances in laser and photonic technology has seen the development of lasers with increasing power and increasingly short pulsewidths, which have become available over an increasing range of wavelengths. As the availability of laser sources grow, so do their applications. To make better use of this improving technology, understanding and controlling laser propagation in free space is critical, as is understanding the interaction between laser light and matter.The need to better control the light obtained from increasingly advanced laser sources leads to the emergence of beam engineering, the systematic understanding and control of light through refractive media and free space. Beam engineering enables control over the beam shape, energy and spectral composition during propagation, which can be achieved through a variety of means. In this dissertation, several methods of beam engineering are investigated. These methods enable improved control over the shape and propagation of laser light. Laser-matter interaction is also investigated, as it provides both a means to control the propagation of pulsed laser light through the atmosphere, and provides a means to generation remote sources of radiation.
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Date Issued: 2013
Identifier: CFE0004650, ucf:49881
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0004650

Title: TOWARDS DIRECT WRITING OF 3-D PHOTONIC CIRCUITS USING ULTRAFAST LASERS.
Creator: Zoubir, Arnaud, Richardson, Martin, University of Central Florida
Abstract / Description: The advent of ultrafast lasers has enabled micromachining schemes that cannot be achieved by other current techniques. Laser direct writing has emerged as one of the possible routes for fabrication of optical waveguides in transparent materials. In this thesis, the advantages and limitations of this technique are explored. Two extended-cavity ultrafast lasers were built and characterized as the laser sources for this study, with improved performance over existing systems. Waveguides are...
Show moreThe advent of ultrafast lasers has enabled micromachining schemes that cannot be achieved by other current techniques. Laser direct writing has emerged as one of the possible routes for fabrication of optical waveguides in transparent materials. In this thesis, the advantages and limitations of this technique are explored. Two extended-cavity ultrafast lasers were built and characterized as the laser sources for this study, with improved performance over existing systems. Waveguides are fabricated in oxide glass, chalcogenide glass, and polymers, these being the three major classes of materials for the telecommunication industry. Standard waveguide metrology is performed on the fabricated waveguides, including refractive index profiling and mode analysis. Furthermore, a finite-difference beam propagation method for wave propagation in 3D-waveguides is proposed. The photo-structural modifications underlying the changes in the material optical properties after exposure are investigated. The highly nonlinear processes of the light/matter interaction during the writing process are described using a free electron model. UV/visible absorption spectroscopy, photoluminescence spectroscopy and Raman spectroscopy are used to assess the changes occurring at the atomic level. Finally, the impact of laser direct writing on nonlinear waveguide applications is discussed.
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Date Issued: 2004
Identifier: CFE0000236, ucf:46252
Format: Document (PDF)
PURL: http://purl.flvc.org/ucf/fd/CFE0000236

laser (5)	+ -
femtosecond (4)	+ -
ultrafast (3)	+ -
ultrafast laser (3)	+ -
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Ultrafast Laser (2)	+ -
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optics (2)	+ -
ultrafast lasers (2)	+ -
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Attosecond science (1)	+ -
Axicon (1)	+ -
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CPA (1)	+ -
Carrier Envelope Phase (1)	+ -
Current Pulses (1)	+ -
DPA (1)	+ -
Diffraction (1)	+ -
EMP (1)	+ -
Electron density (1)	+ -
Energy Projection (1)	+ -
Filament (1)	+ -
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University of Central Florida (17)	+ -
Richardson, Martin (11)	+ -
Delfyett, Peter (7)	+ -
Chang, Zenghu (6)	+ -
Gaume, Romain (3)	+ -

Schulzgen, Axel (3)	+ -
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Chini, Michael (2)	+ -
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