Current Search:  second harmonic generation (x)

View All Items

  • CSV Spreadsheet
(1 - 5 of 5)
QUADRATIC SPATIAL SOLITON INTERACTIONS
Title
QUADRATIC SPATIAL SOLITON INTERACTIONS.
Creator
Jankovic, Ladislav, Stegeman, George I., University of Central Florida
Abstract / Description
Quadratic spatial soliton interactions were investigated in this Dissertation. The first part deals with characterizing the principal features of multi-soliton generation and soliton self-reflection. The second deals with two beam processes leading to soliton interactions and collisions. These subjects were investigated both theoretically and experimentally. The experiments were performed by using potassium niobate (KNBO3) and periodically poled potassium titanyl phosphate (KTP) crystals....
Show moreQuadratic spatial soliton interactions were investigated in this Dissertation. The first part deals with characterizing the principal features of multi-soliton generation and soliton self-reflection. The second deals with two beam processes leading to soliton interactions and collisions. These subjects were investigated both theoretically and experimentally. The experiments were performed by using potassium niobate (KNBO3) and periodically poled potassium titanyl phosphate (KTP) crystals. These particular crystals were desirable for these experiments because of their large nonlinear coefficients and, more importantly, because the experiments could be performed under non-critical-phase-matching (NCPM) conditions. The single soliton generation measurements, performed on KNBO3 by launching the fundamental component only, showed a broad angular acceptance bandwidth which was important for the soliton collisions performed later. Furthermore, at high input intensities multi-soliton generation was observed for the first time. The influence on the multi-soliton patterns generated of the input intensity and beam symmetry was investigated. The combined experimental and theoretical efforts indicated that spatial and temporal noise on the input laser beam induced multi-soliton patterns. Another research direction pursued was intensity dependent soliton routing by using of a specially engineered quadratically nonlinear interface within a periodically poled KTP sample. This was the first time demonstration of the self-reflection phenomenon in a system with a quadratic nonlinearity. The feature investigated is believed to have a great potential for soliton routing and manipulation by engineered structures. A detailed investigation was conducted on two soliton interaction and collision processes. Birth of an additional soliton resulting from a two soliton collision was observed and characterized for the special case of a non-planar geometry. A small amount of spiraling, up to 30 degrees rotation, was measured in the experiments performed. The parameters relevant for characterizing soliton collision processes were also studied in detail. Measurements were performed for various collision angles (from 0.2 to 4 degrees), phase mismatch, relative phase between the solitons and the distance to the collision point within the sample (which affects soliton formation). Both the individual and combined effects of these collision variables were investigated. Based on the research conducted, several all-optical switching scenarios were proposed.
Show less
Date Issued
2004
Identifier
CFE0000090, ucf:46135
Format
Document (PDF)
PURL
http://purl.flvc.org/ucf/fd/CFE0000090
Design of surface chemical reactivity and optical properties in glasses
Title
Design of surface chemical reactivity and optical properties in glasses.
Creator
Lepicard, Antoine, Richardson, Kathleen, Seal, Sudipta, Gaume, Romain, Dussauze, Marc, Kuebler, Stephen, University of Central Florida
Abstract / Description
Thermal poling is a technique which involves the application of a strong DC electric field to a glass substrate heated below its glass transition temperature (Tg). Following the treatment, a static electric field is frozen inside the glass matrix, effectively breaking its centrosymmetry. Historically, this treatment has been used as a way to gain access to second order non-linear optical properties in glasses. However, recent efforts have shown that the treatment was responsible for...
Show moreThermal poling is a technique which involves the application of a strong DC electric field to a glass substrate heated below its glass transition temperature (Tg). Following the treatment, a static electric field is frozen inside the glass matrix, effectively breaking its centrosymmetry. Historically, this treatment has been used as a way to gain access to second order non-linear optical properties in glasses. However, recent efforts have shown that the treatment was responsible for structural changes as well as surface property modifications. Our study was focused on using this technique to tailor surface properties in oxide (borosilicate and niobium borophosphate) and chalcogenide glasses. A strong emphasis was put on trying to control all changes at the micrometric scale. After poling, property changes were assessed using a set of characterization tools: the Maker fringes technique (a Second Harmonic Generation ellipsometry technique), micro-Second Harmonic Generation ((&)#181;-SHG), vibrational spectroscopy and Secondary Ion Mass Spectroscopy (SIMS). Surface reactivity in borosilicate glasses was effectively changed while in niobium borophosphate and chalcogenide glasses, the optical properties were controlled linearly and nonlinearly. Finally, property changes were effectively controlled at the micrometric scale. This opens up new applications of thermal poling as a mean to design glass substrate for integrated photonics and lab-on-a-chip devices.
Show less
Date Issued
2016
Identifier
CFE0006471, ucf:51435
Format
Document (PDF)
PURL
http://purl.flvc.org/ucf/fd/CFE0006471
Nonlinear Dynamics in Multimode Optical Fibers
Title
Nonlinear Dynamics in Multimode Optical Fibers.
Creator
Eftekhar, Mohammad Amin, Christodoulides, Demetrios, Amezcua Correa, Rodrigo, Li, Guifang, Kaup, David, University of Central Florida
Abstract / Description
Multimode optical fibers have recently reemerged as a viable platform for addressing a number of long-standing issues associated with information bandwidth requirements and power-handling capabilities. The complex nature of heavily multimoded systems can be effectively exploited to observe altogether novel physical effects arising from spatiotemporal and intermodal linear and nonlinear processes. Here, we have studied nonlinear dynamics in multimode optical fibers (MMFs) in both the normal...
Show moreMultimode optical fibers have recently reemerged as a viable platform for addressing a number of long-standing issues associated with information bandwidth requirements and power-handling capabilities. The complex nature of heavily multimoded systems can be effectively exploited to observe altogether novel physical effects arising from spatiotemporal and intermodal linear and nonlinear processes. Here, we have studied nonlinear dynamics in multimode optical fibers (MMFs) in both the normal and anomalous dispersion regimes. In the anomalous dispersion regime, the nonlinearity leads to a formation of spatiotemporal 3-D solitons. Unlike in single-mode fibers, these solitons are not unique and their properties can be modified through the additional degrees of freedom offered by these multimoded settings. In addition, soliton related processes such as soliton fission and dispersive wave generation will be also drastically altered in such multimode systems. Our theoretical work unravels some of the complexities of the underlying dynamics and helps us better understand these effects. The nonlinear dynamics in such multimode systems can be accelerated through a judicious fiber design. A cancelation of Raman self-frequency shifts and Blue-shifting multimode solitons were observed in such settings as a result of an acceleration of intermodal oscillations. Spatiotemporal instabilities in parabolic-index multimode fibers will also be discussed. In the normal dispersion regime, this effect can be exploited to generate an ultrabroad and uniform supercontinuum that extends more than 2.5 octaves. To do so, the unstable spectral regions are pushed away from the pump, thus sweeping the entire spectrum. Multimode parabolic pulses were also predicted and observed in passive normally dispersive tapered MMFs. These setting can obviate the harsh bandwidth limitation present in single-mode system imposed by gain medium and be effectively used for realizing high power multimode fiber lasers. Finally, an instant and efficient second-harmonic generation was observed in the multimode optical fibers. Through a modification of initial conditions, the efficiency of this process could be enhanced to a record high of %6.5.
Show less
Date Issued
2018
Identifier
CFE0007399, ucf:52063
Format
Document (PDF)
PURL
http://purl.flvc.org/ucf/fd/CFE0007399
Hybrid integration of second- and third-order highly nonlinear waveguides on silicon substrates
Title
Hybrid integration of second- and third-order highly nonlinear waveguides on silicon substrates.
Creator
Camacho Gonzalez, Guillermo Fernando, Fathpour, Sasan, Likamwa, Patrick, Amezcua Correa, Rodrigo, Peale, Robert, University of Central Florida
Abstract / Description
In order to extend the capabilities and applications of silicon photonics, other materials and compatible technologies have been developed and integrated on silicon substrates. A particular class of integrable materials are those with high second- and third-order nonlinear optical properties. This work presents contributions made to nonlinear integrated photonics on silicon substrates, including chalcogenide waveguides for over an octave supercontinuum generation, and rib-loaded thin-film...
Show moreIn order to extend the capabilities and applications of silicon photonics, other materials and compatible technologies have been developed and integrated on silicon substrates. A particular class of integrable materials are those with high second- and third-order nonlinear optical properties. This work presents contributions made to nonlinear integrated photonics on silicon substrates, including chalcogenide waveguides for over an octave supercontinuum generation, and rib-loaded thin-film lithium niobate waveguides for highly efficient second-harmonic generation. Through the pursuit of hybrid integration of the two types of waveguides for applications such as on-chip self-referenced optical frequency combs, we have experimentally demonstrated fabrication integrability of chalcogenide and thin-film lithium niobate waveguides in a single chip and a pathway for both second- and third-order nonlinearities occurring therein. Accordingly, design specifications for an efficient nonlinear integrated waveguide are reported, showing over an octave supercontinuum generation and frequency selectivity for second-harmonic generation, enabling potentials of on-chip interferometry techniques for carrier-envelope offset detection, and hence stabilized optical combs.
Show less
Date Issued
2019
Identifier
CFE0007607, ucf:52560
Format
Document (PDF)
PURL
http://purl.flvc.org/ucf/fd/CFE0007607
NONLINEAR OPTICAL PROPERTIES OF ORGANIC CHROMOPHORES CALCULATED WITHIN TIME DEPENDENT DENSITY FUNCTIONAL THEORY
Title
NONLINEAR OPTICAL PROPERTIES OF ORGANIC CHROMOPHORES CALCULATED WITHIN TIME DEPENDENT DENSITY FUNCTIONAL THEORY.
Creator
Tafur, Sergio, Kokoouline, Viatcheslav, University of Central Florida
Abstract / Description
Time Dependent Density Functional Theory offers a good accuracy/computational cost ratio among different methods used to predict the electronic structure for molecules of practical interest. The Coupled Electronic Oscillator (CEO) formalism was recently shown to accurately predict Nonlinear Optical (NLO) properties of organic chromophores when combined with Time Dependent Density Functional Theory. Unfortunately, CEO does not lend itself easily to interpretation of the structure activity...
Show moreTime Dependent Density Functional Theory offers a good accuracy/computational cost ratio among different methods used to predict the electronic structure for molecules of practical interest. The Coupled Electronic Oscillator (CEO) formalism was recently shown to accurately predict Nonlinear Optical (NLO) properties of organic chromophores when combined with Time Dependent Density Functional Theory. Unfortunately, CEO does not lend itself easily to interpretation of the structure activity relationships of chromophores. On the other hand, the Sum Over States formalism in combination with semiempirical wavefunction methods has been used in the past for the design of simplified essential states models. These models can be applied to optimization of NLO properties of interest for applications. Unfortunately, TD-DFT can not be combined directly with SOS because state-to-state transition dipoles are not defined in the linear response TD approach. In this work, a second order CEO approach to TD-DFT is simplified so that properties of double excited states and state-to-state transition dipoles may be expressed through the combination of linear response properties. This approach is termed the a posteriori Tamm-Dancoff approximation (ATDA), and validated against high-level wavefunction theory methods. Sum over States (SOS) and related Two-Photon Transition Matrix formalism are then used to predict Two-Photon Absorption (2PA) profiles and anisotropy, as well as Second Harmonic Generation (SHG) properties. Numerical results for several conjugated molecules are in excellent agreement with CEO and finite field calculations, and reproduce experimental measurements well.
Show less
Date Issued
2007
Identifier
CFE0001853, ucf:47372
Format
Document (PDF)
PURL
http://purl.flvc.org/ucf/fd/CFE0001853